化学与材料科学学院

化学与材料科学学院

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盛天

 

     


              

 


盛天   博士


tsheng@ahnu.edu.cn


礼勤楼437


 

个人经历


2014 - 2017,厦门大学,博士后

2011 - 2014,贝尔法斯特女王大学,博士,

2007 - 2011,华东理工大学,学士

 

研究领域


密度泛函计算、理论催化



发表论文


49. F. Liu, C. Chen, X. Jiang, J. Y. Guo, Y. S. Wei, J. W. Li, T. Sheng*, X. S. Zhao*, L. Wei*, High-index surface structure engineering of Au-Pd concave triple-octahedrons for boosting electrocatalytic nitrate reduction to ammonia, ACS Sustainable Chem. Eng., 2023, 11, 1631-1637.

48. F. Zhao, L. Zheng, Q. Yuan*, Q. Zhang, T. Sheng*, X. Yang, L. Gu, X. Wang*, PtCu subnanoclusters epitaxial on PtCu/Pt skin matrix as ultrahigh stable cathode electrocatalysts for room-temperature hydrogen fuel cells, Nano Res., 2023, 16, 2252-2258.

47. Z. Zhang, S. Yang, R. Jiang, T. Sheng*, C. Shi*, Y. Chen*, L. Wang*, Intensifying uneven charge distribution via geometric distortion engineering in atomically dispersed M-Nx/S sites for efficient oxygen electroreduction, Nano Res., 2022, 15, 8928-8935.

46. W. Sun, P. Wang, Y. Jiang, Z. Jiang, R. Long, Z. Chen, P. Song, T. Sheng*, Z. Wu*, Y. Xiong*, V-doped Cu2Se hierarchical nanotubes enabling flow-cell CO2 electroreduction to ethanol with high efficiency and selectivity, Adv. Mater., 2022, 34, 2207691.

45. T. Sheng*, H. Y. Wu, X. Lin, W. F. Lin*, Insights into reaction mechanisms of ethanol electrooxidation at the Pt/Au(111) interfaces by density functional theory, Phys. Chem. Chem. Phys., 2022, 24, 27277.

44. X. Zhou, Y. Mo, F. Yu*, L. Liao, X. Yong, F. Zhang, D. Li, Q. Zhou, T. Sheng*, H. Zhou*, Engneering active iron sites on nanoporous bimetal phosphide/nitride heterostructure array enabling robust overall water splitting, Adv. Funct. Mater., 2022, 2209465.

43. L. Ding, N. Zhu, Y. Hu, Z. Chen, P. Song, T. Sheng*, Z. Wu*, Y. Xiong*, Over 70% Faradaic efficiency for CO2 electroreduction to ethanol enabled by K dopant-tuned Cu sites-intermediates interaction, Angew. Chem. Int. Ed., 2022, 61, e202209268.

42. R. Yun*, B. Zhang, F. Zhan, Z. Xin, T. Sheng*, Z. Shi*, Electrocatalysis CO2 to tunable syngas upon Fe clusters catalyst dispersed on bamboo-like NCTs, Inorg. Chem., 2022, 61, 9375-9380.

41. F. Liu, X. Jiang, H. H. Wang, C. Chen, Y. H. Yang, T. Sheng*, W. S. Wei, X. S. Zhao*, L. Wei*, Boosting electrocatalytic hydrazine oxidation reaction on high-index faceted Au concave trioctahedral nanocrystals, ACS Sustainable Chem. Eng., 2022, 10, 696-702.

40. B. A. Lu, L. F. Shen, J. Liu, Q. Zhang, L. Y. Wan, D. J. Morris, R. X. Wang, Z. Y. Zhou, G. Li, T. Sheng*, L. Gu, P. Zhang, N. Tian*, S. G. Sun*, Structurally disordered phosphorus-doped Pt as a highly active electrocatalyst for an oxygen reduction reaction, ACS Catal., 2021, 11, 355-363.

39. R. Yun*, Z. W. Ma, Y. Hu, F. Zhan, C. Qiu, B. Zheng*, T. Sheng*, Nano-Ni-MOFs: High active catalysts on the cascade hydrogenation of quinolines, Catal. Lett., 2021, 151, 2445-2451.

38. W. Zhang, L. Ding, W. Sun, T. Sheng*, Z. Wu*, F. Gao*, Ultrasmall Pt nanoparticles loaded crystalline MoO2/amorphous Ni(OH)2 hybrid nanofilm with enhanced water dissociation and sufficient hydrogen spillover hydrogen generation, ACS Sustainable Chem. Eng., 2021, 9, 8257-8269.

37. L. N. Chen, S. H. Wang, P. Y. Zhang, Z. X. Chen, X. Lin, H. J. Yang, T. Sheng*, W. F. Lin*, N. Tian, S. G. Sun, Z. Y. Zhou*, Ru nanoparticles supported on partially reduced TiO2 as highly efficient catalyst for hydrogen evolution, Nano Energ., 2021, 88, 106211.

36. R. Yun*, B. Zhang, C. Qiu, Z. Ma, F. Zhan, T. Sheng*, B. Zheng*, Encapsulating cobalt into N-doping hollow frameworks for efficient cascade catalysis, Inorg. Chem., 2021, 60, 9757-9761.

35. C. Qiang, L. Zhang, H. He, Y. Liu, Y. Zhao, T. Sheng*, S. Liu*, X. Wu, Z. Fang*, Efficient electrocatalytic water splitting by bimetallic cobalt iron boride nanoparticles with controlled electronic structure, J. Colloid Interface Sci., 2021, 645, 650-659.

34. L. Gao. T. Sheng*, M. Wang, H. Ren, S. W. Joo*, J. Huang*, Titanium nitride nanocrystals anchored evenly on interconnected carbon nanosheets with effective chemisorption and catalytic effects towards polysulfides for long-life lithium-sulfur batteries, Electrochim. Acta, 2021, 395, 139208.

33. L. Wei*, F. Liu, X. Jiang, Y. H. Yang, T. Sheng*, Q. Q. Xu, X. S. Zhao, Y. J. Fan*, High-index faceted Pt-Ru alloy concave nanocubes with enhancing ethanol and CO electro-oxidation, Electrochim. Acta, 2021, 396, 139266.

32. Q. S. Chen*, J. X. Tang, Z. N. Xu, T. Sheng*, G. C. Guo*, Shape-dependent catalytic properties of electrochemically synthesized PdPt nanoparticles towards alcohols electrooxidation, J. Electroanal. Chem., 2021, 896, 115189.

31. Y. J. Mao, F. Liu, Y. H. Chen, X. Jiang, X. S. Zhao, T. Sheng*, J. Y. Ye, H. G. Liao, L. Wei*, S. G. Sun*, Enhancing electrocatalytic nitrogen reduction to ammonia with rare earth (La, Y and Sc) on high-index faceted platinum alloy concave nanocubes, J. Mater. Chem. A, 2021, 9, 26277-26285.

30. Z. Huang, R. Wang, T. Sheng*, X. Zhong, S. Wang*, X. Zhu, Q. Yuan, Y. Wei, S. Zhou, Transformation of the sp2 carbanion to carbene with subsequent 1,1-migratory insertion and nucleophilic substitution in rate-earth metal chemistry, Inorg. Chem., 2021, 60, 18843-18853.

29. T. Sheng*, Zi-Wei Ma, S. G. Sun*, Insights into the Pt/Rh(111) interface for direct ethanol fuel cells, Appl. Surf. Sci., 2020, 502, 144093.

28. H. Xu, W. Zhang, J. Zhang, Z. Wu*, T. Sheng*, F. Gao*, An Fe-doped Co11(HPO3)8(OH)6 nanosheets array for high-performance water electrolysis, Electrochim. Acta, 2020, 334, 135616.

27. Y. C. Wang, L. Y. Wan, P. X. Cui, L. Tong, Y. Q. Ke, T. Sheng*, M. Zhang, S. H. Sun*, H. W. Liang, Y. S. Wang, K. Zaghib, Z. Y. Zhou, J. Y. Yuan*, Porous carbon-membrane supported pyrrole-type Fe-N4 as active sites for electrochemical hydrazine oxidation reaction, Small, 2020, 16, 2002203.

26. R. Yun*, F. Zhan, J. Ma, L. Hong, B. Zhang, T. Sheng*, B. Zheng*, Fe single atoms and Fe2O3 clusters liberating from N-doped polyhedral carbon for chemo-selectivity hydrogenation under mild conditions, ACS Appl. Mater. Inter., 2020, 12, 34122-34129.

25. T. Sheng*, C. Qiu, X. Lin, W. F. Lin*, S. G. Sun*, Insights into ethanol electro-oxidation over solvated Pt(100): Origin of selectivity and kinetics revealed by DFT, Appl. Surf. Sci., 2020, 553, 147505.

24. Y. C. Jiang, Y. J. Mao, J. Zou, H. H. Wang, F. Liu, Y. S. Wei, T. Sheng*, X. S. Zhao, L. Wei*, Electrochemically shape-controlled synthesis of great stellated dodecahedral Au nanocrystals with high-index facets for nitrogen reduction to ammonia, Chem. Commun., 2020, 56, 12612-12615.

23. X. Zhu*, D. Guo, Z. Huang, T. Sheng*, S. Wang*, M. Pan, L. Zha, S. Zhou, Dehydrogenative coupling of terminal alkynes with O/N-based monohydrosilanes catalysed by rare-earth metal complexes, Inorg. Chem., 2020, 59, 19, 14152-14161.

22. B. W. Zhang#, T. Sheng# (co-first author), Y. X. Wang*, S. L. Chou, K. Davey, S. X. Dou, S. Z. Qiao*, Long-life room-temperature sodium-sulfur batteries by virtue of transition metal nanocluster-sulfur interactions, Angew. Chem. Int. Ed., 2019, 58, 1484-1488.

21. L. F. Shen, B. A. Lu, X. M. Qu, J. Y. Ye, J. M. Zhang, S. H. Yin, Q. H. Wu, R. X. Wang, S. Y. Shen, T. Sheng*, Y. X. Jiang*, S. G. Sun*, Does the oxophilic effect serve the same role for hydrogen evolution/oxidation reaction in alkaline media? Nano Eneng., 2019, 62, 601-609.

20. Y. J. Mao, L. Wei*, X. S. Zhao, Y. S. Wei, J. W. Li, T. Sheng*, F. C. Zhu, N. Tian, Z. Y. Zhou, S. G. Sun*, Excavated cubic platinum-iridium alloy nanocrystals with high-index facets as highly efficient electrocatalyst in N2 fixation to NH3, Chem. Commun., 2019, 55, 9335-9338.

19. L. Wei, Y. J. Mao, F. Liu, T. Sheng*, Y. S. Wei, J. W. Li, Y. J. Fan*, X. S. Zhao*, Concave cubic Pt-Sm alloy nanocrystal with high-index facets and enhanced electrocatalytic ethanol oxidation, ACS Appl. Energ. Mater., 2019, 2, 7204-7210.

18. S. Xu, W. Hou, R. Jiang, L. Li, T. Sheng*, L. Wang*, Regulating location of active sites: a novel strategy to greatly improve stability of PtAu electrocatalysts, Chem. Commun., 2019, 55, 13602-13605.

17. D. Wang#, T. Sheng# (co-first author), J. F. Chen, H. F. Wang*, P. Hu*, Identifying the key obstacle in photocatalytic oxygen evolution on rutile TiO2, Nat. Catal., 2018, 1, 291-299.

16. G. L. Xu#, L. Xiao#, T. Sheng# (co-first author), J. Liu, Y. X. Hu, T. Ma, R. Amine, Y. Xie, X. Zhang, Y. Liu, Y. Ren, C. J. Sun, S. M. Heald, J. Kovacevic, Y. H. Sehlleier, C. Schulz, W. L. Mattis, S. G. Sun, H. Wiggers, Z. Chen, K. Amine, Electrostatic self-assembly enabling integrated bulk and interfacial sodium storage in 3D titania-graphene hybrid, Nano Lett., 2018, 18, 336-346.

15. T. Sheng*, S. G. Sun, Modelling the aqueous and nonaqueous interfaces for CO2 electro-reduction over Sn catalysts, Appl. Surf. Sci., 2018, 428, 514-519.

14. T. Sheng*, S. G. Sun, Electrochemical reduction of CO2 into CO on Cu(100): a new insight into the C-O bond breaking mechanism, Chem. Commun., 2017, 53, 2594-2597.

13. T. Sheng*, J. Y. Ye, W. F. Lin, W. S. G. Sun*, An insight into methanol oxidation mechanisms on RuO2(100) under an aqueous environment by DFT calculations, Phys. Chem. Chem. Phys., 2017, 19, 7476-7480.

12. T. Sheng, N. Tian, Z. Y. Zhou, W. F. Lin, S. G. Sun*, Designing Pt-based electrocatalyts with high surface energy, ACS Energ. Lett., 2017, 2, 1892-1900.

11. T. Sheng*, S. G. Sun, Identifying the significance of proton-electron transfer in CH4 formation on Cu(100) during CO2 electro-reduction, J. Electroanal. Chem., 2017, 793, 184-187.

10. T. Sheng*, S. G. Sun, Free energy landscape of electrocatalytic CO2 reduction to CO on aqueous FeN4 center embedded graphene studied by ab initio molecular dynamics simulations, Chem. Phys. Lett., 2017, 688, 37-42.

9. T. Sheng, Y. F. Xu, Y. X. Jiang, L. Huang, N. Tian, Z. Y. Zhou, I. Broadwell, S. G. Sun*, Structure design and performance tuning of nanomaterials for electrochemical energy conversion and storage, Acc. Chem. Res., 2016, 49, 2569-2577.

8. T. Sheng, Y. J. Qi, X. Lin, P. Hu, S. G. Sun, W. F. Lin*, Insights into the mechanism of nitrobenzene reduction to aniline over Pt catalyst and the significance of the adsorption of phenyl group on kinetics, Chem. Eng. J., 2016, 293, 337-344.

7. T. Sheng*, D. Wang, W. F. Lin, P. Hu, S. G. Sun*, Insight into CO activation over Cu(100) under electrochemical conditions, Electrochim. Acta, 2016, 190, 446-454.

6. T. Sheng*, W. F. Lin, S. G. Sun*, Elucidation of the surface structure-selectivity relationship in ethanol electro-oxidation over platinum by density functional theory, Phys. Chem. Chem. Phys., 2016, 18, 15501-15504.

5. T. Sheng*, W. F. Lin, S. G. Sun*, Electrochemical interfacial influences on deoxygenation and hydrogenation reactions in CO reduction on a Cu(100) surface, Phys. Chem. Chem. Phys., 2016, 18, 15304-15311.

4. T. Sheng*, S. G. Sun*, Insight into the promoting role of Rh doped on Pt(111) in methanol electro-oxidation, J. Electroanal. Chem., 2016, 781, 24-29.

3. T. Sheng, X. Lin, Z. Y. Chen, P. Hu, S. G. Sun, Y. Q. Chu, C. A. Ma, W. F. Lin*, Methanol electro-oxidation on platinum modified tungsten carbides in direct methanol fuel cells: a DFT study, Phys. Chem. Chem. Phys., 2015, 17, 25235-25243.

2. T. Sheng, W. F. Lin*, C. Hardacre, P. Hu*, Significance of beta-dehydrogenation in ethanol electro-oxidation on platinum doped with Ru, Rh, Pd, Os and Ir, Phys. Chem. Chem. Phys., 2014, 16, 13248-13254.

1. T. Sheng, W. F. Lin*, C. Hardacre, P. Hu*, Role of water and adsorbed hydroxyls on ethanol electrochemistry on Pd: new mechanism, active centers, and energetics for direct ethanol fuel cell running in alkaline medium, J. Phys. Chem. C, 2014, 118, 5762-5772.

 

 

 

 

 


编辑:盛天   |   更新日期:2019-03-07   |   点击:5739
 

 


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